张大帅

男， 德州学院化学化工学院， 教授/研究员/教授级高工或同等级别

学习/工作经历

2005.09—2009.06，聊城大学化学化工学院化学专业学习，获理学学士学位；
2009.09—2014.06，南开大学化学学院物理化学专业学习（硕博连读），获理学博士学位；
2014.06—2018.12，德州学院化学化工学院学院讲师；
2019.01—2024.12，德州学院化学化工学院学院副教授；
2023.09—2024.08，南开大学访问学者；
2025.01—至今，德州学院化学化工学院教授。

研究领域和兴趣

功能金属有机框架材料

主要业绩

张大帅，博士毕业于南开大学化学学院物理化学专业，现为德州学院化学化工学院教授/硕士生导师，担任山东化学化工学会无机化学专业委员会委员，入选德州市B类国家级领军人才，主要从事金属有机框架及其衍生功能材料研究。近年来，以吸附分离、催化、发光功能为导向，系统研究了高性能MOF的构筑策略及性能调控方法；率先利用调控配体柔性、精准控制微环境等策略，成功构建高稳定MOF材料体系，并发展了混合相MOF的纯化技术，为突破MOF的应用瓶颈提供了独特方案；将给-受体体系定向引入MOF实现了给-受体材料的功能导向精准构筑，并进一步实现了给-受体MOF的抗热猝灭发光，对该领域的发展做出原创性贡献。先后主持国家自然科学青年基金项目、山东省高校青创人才引育计划项目（200万）等项目。发表论文70余篇，其中以第一或通讯作者在Adv. Mater.、Mater. Horiz.、ACS Appl. Mater. Interfaces、Chin. Chem. Lett.等发表高水平论文30篇（高被引1篇、热点论文2篇），成果得到国内外学者正面引用2100余次。以第一发明人授权发明专利2件、软件著作权1件，指导本科生授权发明专利1项。以第一完成人获得中国有色金属工业协会科技进步奖二等奖、德州市自然科学优秀成果奖一等奖(2项)；以主要完成人获得中国商业联合会服务业科技创新二等奖、中国石化联合会科技进步奖三等奖、山东省高校科技奖三等奖（2项）、山东省材料学会科技成果奖三等奖等奖项。

代表成果

1. Da-Shuai Zhang#, Qiang Gao#, Ze Chang, Xiao-Ting Liu, Bei Zhao, Zhi-Hong Xuan, Tong-Liang Hu, Ying-Hui Zhang, Jian Zhu, Xian-He Bu, Rational Construction of Highly Tunable Donor–Acceptor Materials Based on a Crystalline Host–Guest Platform. Advanced Materials, 2018, 30, 1804715. DOI: 10.1002/adma.201804715.
2. Yong-Zheng Zhang, Xiang-Jing Kong, Wen-Feng Zhou, Chun-Hui Li, Hui Hu, Hengnuo Hou, Zhongmin Liu, Longlong Geng,* Hongliang Huang,* Xiuling Zhang, Da-Shuai Zhang,* and Jian-Rong Li, Pore Environment Optimization of Microporous Metal−Organic Frameworks with Huddled Pyrazine Pillars for C2H2/CO2 Separation. ACS Applied Materials & Interfaces, 2023, 15, 4208-4215. DOI: 10.1021/acsami.2c19779.
3. Da-Shuai Zhang, Yong-Zheng Zhang, Xiuling Zhang*, Fei Wang, Jian Zhang, Hui Hu, Jun Gao, Hui Yan, Hui-Ling Liu, Hui-Yan Ma, Long-Long Geng, Yun-Wu Li*, Nanocage-Based Porous Metal–Organic Frameworks Constructed from Icosahedrons and Tetrahedrons for Selective Gas Adsorption. ACS Applied Materials & Interfaces, 2019, 11, 20104-20109. DOI: 10.1021/acsami.9b05655.
4. Xiuling Zhang#, Yongzheng Zhang#, Wenfeng Zhou, Huiling Liu, Dashuai Zhang*, Hui Hu, Chao Lv, Suijun Liu*, Longlong Geng*, Construction of novel cluster-based MOF as multifunctional platform for CO2 catalytic transformation and dye selective adsorption. Chinese Chemical Letters, 2023, 34, 107368. DOI: 10.1016/j.cclet.2022.03.091.
5. Longlong Geng, Huiling Liu, Wenfeng Zhou, Yong-Zheng Zhang,* Hongliang Huang, Da-Shuai Zhang,* Hui Hu, Chao Lv, Xiuling Zhang, Suijun Liu,* Construction of metal-organic frameworks with unsaturated Cu sites for efficient and fast reduction of nitroaromatics: A combined experimental and theoretical study. Chinese Chemical Letters, 2024, 35, 109120. DOI: 10.1016/j.cclet.2023.109120.
6. Zhen-Wei Zhang#, Da-Shuai Zhang#*, Wei Wang, Xiao-Ting Liu, Hui Hu, Yong-Zheng Zhang, Longlong Geng, Bin Li, Yuchen Deng, Rongmin Wei, Xiuling Zhang, Yuexing Zhang*, Ze Chang*, Construction of through-space charge transfer donor-acceptor coordination polymers through the combination of planar electron-deficient/rich ligands. Chinese Chemical Letters, 2025, 110710. DOI: 10.1016/j.cclet.2024.110710.
7. Da-Shuai Zhang,*† Zhen-Wei Zhang,† Wei Wang, Xiao-Ting Liu, Qiang Gao, Jingjing Pang, Yong-Zheng Zhang, Longlong Geng, Chuanqi Feng, Yanyan Gao, Sha Sha, Ai-Yun Ni, Bin Li, Xiuling Zhang, Hui Hu,* and Ze Chang*, Rare-earth-based donor-acceptor metal-organic frameworks with low thermal quenching and dual emission mechanisms for high-temperature sensing. Materials Horizons, 2025 , Advance Article. DOI: 10.1039/D5MH00689A.
8. Yong-Zheng Zhang#, Xin-Dan Zhang#, Yan-Kai Zhang, Fu-Tian Wang, Longlong Geng,* Hui Hu, Zhen Li, Da-Shuai Zhang*, Hongliang Huang* and Xiuling Zhang, Linker engineering in mixed-ligand metal–organic frameworks for simultaneously enhanced benzene adsorption and benzene/cyclohexane separation. Inorganic Chemistry Frontiers, 2024, 11, 8101-8109. DOI: 10.1039/D4QI01796J.
9. Da-Shuai Zhang*#, Zhen-Wei Zhang#, Fan-Cui Li, Hongliang Huang, Hui Hu, Yong-Zheng Zhang, Longlong Geng, Rongmin Wei, Xiuling Zhang, Wei Li*, Yun-Wu Li*, Construction of Coordination Spaces with Narrow Pore Windows in Co-Based Metal–Organic Frameworks toward CO2/N2 Separation. Inorganic Chemistry, 2024, 63, 15915-15923. DOI: 10.1021/acs.inorgchem.4c02251.
10. Xiuling Zhang, Ran-Hui Zhang, Hui Hu, Longlong Geng, Yong-Zheng Zhang, Jun Gao, Da-Shuai Zhang*, Yao-Qiang Jin and Jianmin Sheng, Combining unsaturated metal sites and narrow pores within a Co(II)-based MOF towards CO2 separation and transformation. Dalton Transactions, 2020, 49, 2058-2062. DOI: 10.1039/C9DT04736K.

*以上信息由高级会员个人更新和维护。